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Jolie next appeared as the eponymous character in the 2010 thriller Salt, her first film in two years. She starred alongside Liev Schreiber as CIA agent Evelyn Salt, who goes on the run after she is accused of being a KGB sleeper agent. Originally written as male, the character Salt underwent a gender change after a Colombia Pictures executive suggested Jolie for the role to director Phillip Noyce. Salt grossed 293 million worldwide and received generally favorable reviews, with Empire remarking that "when it comes to selling incredible, crazy, death-defying antics, Jolie has few peers in the action business.Later that year, she co-starred with Johnny Depp in The Tourist, directed by Florian Henckel von Donnersmarck. Despite a mostly negative critical reception, the film grossed $268 million worldwide and garnered Jolie a controversial nomination for the Golden Globe Award for Best Actress – Motion Picture Musical or Comedy
Humanitarian work

Jolie first became personally aware of worldwide humanitarian crises while filming Tomb Raider in Cambodia. She eventually turned to for more information on international trouble spots. In order to learn more about the situation and the conditions in these areas, she began visiting refugee camps around the world. In February 2001, Jolie went on her first field visit, an 18-day mission to Sierra Leone and Tanzania; she later expressed her shock at what she had witnessed In the following months, she returned to Cambodia for two weeks and later met with Afghan refugees in Pakistan, where she donated $1 million for Afghan refugees in response to an international emergency appeal She insisted on covering all costs related to her missions and shared the same rudimentary working and living conditions as UNHCR field staff on all of her visits.[52] Jolie was named a Goodwill Ambassador on August 27, 2001 at headquarters in Geneva.

"We cannot close ourselves off to information and ignore the fact that millions of people are out there suffering. I honestly want to help. I don't believe I feel differently from other people. I think we all want justice and equality, a chance for a life with meaning. All of us would like to believe that if we were in a bad situation someone would help us."
Jolie on her motives for joining UNHCR in 2001

Jolie has been on field missions around the world and met with refugees and internally displaced persons in more than 20 countries. Asked what she hoped to accomplish, she stated, "Awareness of the plight of these people. I think they should be commended for what they have survived, not looked down upon. In 2002, Jolie visited the Tham Hin refugee camp in Thailand and Colombian refugees in Ecuador. Jolie later went to various UNHCR facilities in Kosovo and paid a visit to Kakuma refugee camp in Kenya with refugees mainly from Sudan. She also met with Angolan refugees while filming Beyond Borders in Namibia.

In 2003, Jolie embarked on a six-day mission to Tanzania where she traveled to western border camps hosting Congolese refugees, and she paid a week-long visit to Sri Lanka, meeting Tamil refugee orphans in Jaffna. She later concluded a four-day mission to Russia as she traveled to North Caucasus. Concurrently with the release of her movie Beyond Borders, she published Notes from My Travels, a collection of journal entries that chronicle her early field missions (2001-2002). During a private stay in Jordan in December 2003, she asked to visit Iraqi refugees in Jordan's eastern desert and later that month she went to Egypt to meet Sudanese refugees.

On her first U.N. trip within the United States, in 2004, Jolie went to Arizona, visiting detained asylum seekers at three facilities and the Southwest Key Program, a facility for unaccompanied children in Phoenix. She flew to Chad in June 2004, paying a visit to border sites and camps for refugees who had fled fighting in western Sudan's Darfur region. Four months later she returned to the region, this time going directly into West Darfur. Also in 2004, Jolie met with Afghan refugees in Thailand and on a private stay to Lebanon during the Christmas holidays, she visited UNHCR's regional office in Beirut, as well as some young refugees and cancer patients in the Lebanese capital

In 2005, Jolie went to Pakistan to visit Afghani refugees; she also met with Pakistan's President Pervez Musharraf and Prime Minister Shaukat Aziz. She returned to Pakistan with Brad Pitt during the Thanksgiving weekend in November to see the impact of the 2005 Kashmir earthquake. In 2006, Jolie and Pitt flew to Haiti and visited a school supported by Yéle Haïti, a charity founded by Haitian-born hip hop musician Wyclef Jean. While filming A Mighty Heart in India, Jolie met with Afghan and Burmese refugees in New Delhi. She spent Christmas Day 2006